Αρχειοθήκη ιστολογίου

Τετάρτη 12 Δεκεμβρίου 2018

Vinylidenation of Organoboronic Esters Enabled by a Pd‐Catalyzed Metallate Shift

Angewandte Chemie International Edition Vinylidenation of Organoboronic Esters Enabled by a Pd‐Catalyzed Metallate Shift

α‐Methylene organoboronic esters: These compounds are prepared in a catalytic fashion for precursor boronic esters by a Pd‐catalyzed rearrangement of the derived "ate" complexes.


Abstract

Organoboron "ate" complexes undergo a net vinyl insertion reaction to give 1,1‐disubstituted alkenyl boronic esters when treated with stoichiometric allyl acetate and a palladium catalyst. Reactions that employ vinyllithium afforded good to excellent yields after one hour, while reactions that employ vinylmagnesium chloride furnished modest to good yields after 18 hours.



from A via a.sfakia on Inoreader https://ift.tt/2qQ5hOs

Δεν υπάρχουν σχόλια:

Δημοσίευση σχολίου

Medicine by Alexandros G. Sfakianakis,Anapafseos 5 Agios Nikolaos 72100 Crete Greece,00302841026182,00306932607174,alsfakia@gmail.com,

Αναζήτηση αυτού του ιστολογίου

! # Ola via Alexandros G.Sfakianakis on Inoreader